The Values section of css-align currently says:
This specification follows the CSS property definition conventions from [CSS2]. Value types not defined in this specification are defined in CSS Level 2 Revision 1 [CSS2].
I think the section this points to has become sufficiently out-of-date by this point that it's probably best to point mostly to the relevant level 3 modules rather than level 2. Most drafts don't have a section like this one, and I don't think such a section would be needed if bikeshed implemented speced/bikeshed#617